We visited Great Sand Dunes National Park at Labor Day long weekend in 2012. The main feature of the park is, of course, sand dunes. We did an overnight backpacking trip to stay among the dunes. After we set up the tent, we hiked High Dune and waited for sunset. There was a time weather became extremely windy. Wind blew the sand up vigorously. When the sand hit our skin it was really hurt.
On next day, we got up at around 5 AM, then hiked up to wait for sunrise. After sunrise, while temperature was still low, we hiked Star Dune, which is known as the tallest dune in North America. The hike was not too far but it was very strenuous. Do not underestimate it. People usually day-hike to High Dune, then return. During our stay, we did not see anyone hiked Star Dune.

The best sunrise and sunset spots are on top of the dunes. If you do not want to hike, along the paved road, visitor center provides good view for sunset. But it is not nearly as good as being on top of dunes. During our stay, I also waited for sunrise at visitor center but it did not impress me because in early morning the sun was blocked by the mountains surrounding the area.
We also hiked Mosca Pass Trail but we were not impressed.

Sunset | The photo was taken at visitor center

Sun Beams | The photo was taken on top of High Dune at about half hour before sunset.

Wave | The last light before sunset.

Sunset

Sunrise

Sunrise

Rainbow on Sand Dunes | The photo was taken in early morning, on the way to Star Dune.

Sand Dunes and Shadows

Sand Dunes

Top of Star Dune | The tallest dune in North America.

Sunset at countryside

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